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The ORCA output file is your best friend. It contains a wealth of information about what went wrong. Look for error messages, warnings, and any clues about why the SCF failed. Read the output from top to bottom. Things like the number of SCF cycles performed and the energy changes in each cycle are essential pieces of information for diagnosing the problem. Check the end of your output file for specific messages. ORCA often provides very helpful clues about what's gone wrong, such as suggestions on how to improve the calculation, along with error codes that are used to debug. It might tell you which specific step of the SCF procedure failed or provide insights into the nature of the problem, such as the initial guess being too far off or a problem with the geometry.
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